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Well, you'd have to save off the current disk contents and reload onto the raid0. Performance depends on what is implementing the raid0. It's hard to say generally, but roughly 2X? I'd be scare to stripe two disks though, unless I didn't scare about the system - if either dies you're hosed. On the other hand, a raid1 often gives you close to 2X the read speed (depending on how the HW works...)
Would putting another WD 640GB Black in RAID 0 provide a noticeable decrease in boot and loading times and what read and write times should I expect?
I'm not too familiar with RAID but what is the difference between the two?