Is it possible to limit access to a share to local only?

Information is sorely lacking. What exactly are you trying to do/not do?
 
If a user isn't connect to the LAN (local Area Network he/she cannot access the share. In other words, no access from the Internet and beyond. Local access only.
 
Assuming you have a hardware firewall, drop all packets from that device.
 
The simple answer is that you don't allow outside access to the LAN itself. But I assume you're asking this because you intend to let people onto your network for some reason.

It's relatively simple to set up access rights by user account or group.
 
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