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CPU Bound:
WoW
Valve Games
GTA4
GPU Bound:
Everything else
CPU Bound:
WoW
Valve Games
GTA4
GPU Bound:
Everything else
CPU Bound:
WoW
Valve Games
GTA4
BFBC2
GPU Bound:
Everything else
I doubled my frame rates in GTA4 when I upgraded my CPU, then doubled my frame rates again when I upgraded my GPU. So I think it's limited by both.
It's very subjective though. You are a lot more likely to be CPU limited running GTX580 SLI than running a 8800GT.
One game I would put distinctly in the CPU-limited category is Flight Simulator X, but it's basically limited to clock speed and performance per mhz, since it only uses 2 cores.